By Stuart A. Rice, Aaron R. Dinner
The Advances in Chemical Physics series?the innovative of analysis in chemical physics
The Advances in Chemical Physics sequence offers the chemical physics box with a discussion board for severe, authoritative reviews of advances in each quarter of the self-discipline. jam-packed with state-of-the-art learn pronounced in a cohesive demeanour no longer discovered in different places within the literature, every one quantity of the Advances in Chemical Physics sequence serves because the excellent complement to any complex graduate classification dedicated to the learn of chemical physics.
This quantity explores:
Quantum Dynamical Resonances in Chemical Reactions: From A + BC to Polyatomic platforms (Kopin Liu)
The Multiscale Coarse-Graining procedure (Lanyuan Lu and Gregory A. Voth)
Molecular Solvation Dynamics from Inelastic X-ray Scattering Measurements (R.H. Coridan and G.C.L. Wong)
Polymers below Confinement (M. Muthukumar)
Computational reviews of the houses of DNA-linked Nanomaterials (One-Sun Lee and George C. Schatz)
Nanopores: Single-Molecule Sensors of Nucleic Acid dependent Complexes (Amit Meller)
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Extra resources for Advances in Chemical Physics, Volume 149
108, 957 (2010). J. Zhou, J. J. Lin, and K. Liu, J. Chem. , 121, 813 (2004). A. J. Bray and M. A. Moore, Phys. Rev. , 49, 1545 (1982). A. Schmid, Phys. Rev. , 51, 1506 (1983). S. Chakravarty and A. Leggett, Phys. Rev. , 52, 5 (1984). S. A. Rice and P. Gaspard, Israel. J. , 30, 23 (1990). 76. M. Gruebele, Adv. Chem. , 114, 193 (2000). 77. J. Jortner and R. D. Levine, Israel J. , 30, 207 (1990). 78. 79. 80. 81. 82. K. K. Lenmann, G. Scoles, and B. H. Pate, Annu. Rev. Phys. , 45, 241 (1994). D. J.
It is not clear a priori if they are generally applicable to other reactions involving a quantum 24 kopin liu dynamical resonance. Nevertheless, we conjectured that they may be the most incisive and universal indicators in that the observation of both characteristic features strongly suggests the presence of a resonance; though the reverse does not necessarily hold. It should be stressed that the detailed appearances of these resonance features would certainly be different for different reactions; yet, only the general characteristic patterns are of concern here.
17 is the ratio of the REMPI intensities of the two bands, 111 and 000 , as a function of collisional energies. Compared to the ground state methyl products, the formation of CH3 (v1 = 1) is signiﬁcant only at Ec < 1 kcal/mol. Also shown in the inset of Fig. 17 is the reactive excitation function of F + CH4 → CH3 (v = 0) + HF(all v ) . Combining these two results, one can conclude that the reaction of F + CH4 → CH3 (v1 = 1) + HF occurs only near the reaction threshold, which is indeed a quite remarkable observation.